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The Collaborative International Dictionary of English v.0.48:

Unhead \Un*head"\, v. t. [1st pref. un- + head.] [1913 Webster] 1. To take out the head of; as, to unhead a cask. [1913 Webster] 2. To decapitate; to behead. [Obs.] --T. Brown. [1913 Webster]