The Collaborative International Dictionary of English v.0.48:

Calligraphic \Cal`li*graph"ic\, Calligraphical
\Cal`li*graph"ic*al\, a., [Gr. ???????????; pref. ?????- (fr.
   kalo`s beautiful) + gra`fein to write; cf. F.
   calligraphique.]
   Of or pertaining to calligraphy.
   [1913 Webster]

         Excellence in the calligraphic act.      --T. Warton.
   [1913 Webster]

WordNet (r) 3.0 (2006):

calligraphic
    adj 1: of or relating to or expressed in calligraphy [syn:
           calligraphic, calligraphical]