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The Collaborative International Dictionary of English v.0.48:

Attune \At*tune"\, v. t. [imp. & p. p. Attuned; p. pr. & vb. n. Attuning.] [Pref. ad- + tune.] [1913 Webster] 1. To tune or put in tune; to make melodious; to adjust, as one sound or musical instrument to another; as, to attune the voice to a harp. [1913 Webster] 2. To arrange fitly; to make accordant. [1913 Webster] Wake to energy each social aim, Attuned spontaneous to the will of Jove. --Beattie. [1913 Webster]