The Collaborative International Dictionary of English v.0.48:
Alliterate \Al*lit"er*ate\, v. t. To employ or place so as to make alliteration. --Skeat. [1913 Webster]The Collaborative International Dictionary of English v.0.48:
Alliterate \Al*lit"er*ate\, v. i. To compose alliteratively; also, to constitute alliteration. [1913 Webster]WordNet (r) 3.0 (2006):
alliterate v 1: use alliteration as a form of poetry